| 01. | Bleeker Street | 2:42 |
| 02. | The Sound of Silence | 3:05 |
| 03. | The Sun is Burning | 2:46 |
| 04. | Wednesday Morning, 3 a.m. | 2:14 |
| 05. | He Was My Brother | 2:49 |
| 06. | Sparrow | 2:47 |
| 07. | Peggy-O | 2:25 |
| 08. | Benedictus | 2:38 |
| 09. | Somewhere They Can't Find Me | 2:34 |
| 10. | We've Got a Groovy Thing Goin' | 1:57 |
| 11. | Leaves That Are Green | 2:20 |
| 12. | Richard Cory | 2:55 |
| 13. | I Am a Rock | 2:49 |
| 14. | The Sound of Silence (single version) | 3:05 |
| 15. | Homeward Bound | 2:29 |
| 16. | Blues Run the Game | 2:51 |
| 17. | Kathy's Song | 3:17 |
| 18. | April Come She Will | 1:49 |
| 19. | Flowers Never Bend with the Rainfall | 2:10 |
| 20. | Patterns | 2:49 |
| 21. | Cloudy | 2:21 |
| 22. | The Dangling Conversation | 2:37 |
| 23. | (Are You Going To) Scarborough Fair/Canticle | 3:10 |
| 24. | The 59th Street Bridge Song (Feelin' Groovy) | 1:53 |
| 25. | For Emily, Whenever I May Find Her | 2:05 |
| 26. | 7 O'Clock News/Silent Night | 2:03 |
| 27. | A Hazy Shade of Winter | 2:17 |
| 28. | At the Zoo | 2:23 |
| 29. | A Poem on the Underground Wall (live) | 4:30 |
| 30. | Red Rubber Ball (live) | 2:29 |
| 31. | Blessed (live) | 3:40 |
| 32. | Anji (live) | 2:29 |
| 33. | A Church Is Burning (live) | 3:27 |
| 34. | Fakin' It | 3:17 |
| 35. | Save the Life of My Child | 2:49 |
| 36. | America | 3:36 |
| 37. | You Don't Know Where Your Interests Lie | 2:19 |
| 38. | Punky's Dilemma | 2:13 |
| 39. | Comfort and Joy | 1:49 |
| 40. | Star Carol | 1:46 |
| 41. | Mrs. Robinson | 4:03 |
| 42. | Old Friends/Bookends | 3:56 |
| 43. | Overs (live) | 3:05 |
| 44. | A Most Peculiar Man (live) | 2:35 |
| 45. | Bye, Bye Love (live) | 2:44 |
| 46. | The Boxer | 5:08 |
| 47. | Baby Driver | 3:15 |
| 48. | Why Don't You Write Me | 2:46 |
| 49. | Feuilles-O | 1:42 |
| 50. | Keep the Customer Satisfied | 2:35 |
| 51. | So Long, Frank Lloyd Wright | 3:41 |
| 52. | Song for the Asking | 1:49 |
| 53. | Cecilia | 2:55 |
| 54. | El Condor Pasa (If I Could) | 3:06 |
| 55. | Bridge Over Troubled Water | 4:53 |
| 56. | The Only Living Boy in New York | 3:58 |
| 57. | Hey, Schoolgirl/Black Slacks (live) | 1:32 |
| 58. | That Silver Haired Daddy of Mine (live) | 3:26 |
| 59. | My Little Town | 3:51 |